Harder metals get a bigger drill, so the tap works less hard.
For 1/4-20 in aluminum, brass, plastics, use #7 (0.2010 in, 5.11 mm). It leaves about 75% thread, right on the 75% target.
No #7? The closest metric drill is 5.1 mm (0.2008 in), about 76% thread.
Full 1/4-20 tap drill page
Turn on JavaScript to change the thread, material or drill. The tables below work without it.
TapDrillSize: full tap drill charts and thread pages